 Bing CrosbyNarrator (segment "The Legend of Sleepy Hollow") | Narrator (segment "The Legend of Sleepy Hollow") |
 Basil RathboneNarrator (segment "The Wind in the Willows") | Narrator (segment "The Wind in the Willows") |
 Eric BloreMr. Toad (voice) | Mr. Toad (voice) |
 J. Pat O'MalleyCyril Proudbottom (voice) | Cyril Proudbottom (voice) |
| JJohn McLeishProsecutor (voice) | Prosecutor (voice) |
 Colin CampbellMole (voice) | Mole (voice) |
| CCampbell GrantAngus MacBadger (voice) | Angus MacBadger (voice) |
| CClaud AllisterRat (voice) | Rat (voice) |
| OOliver WallaceGang Leader (voice) | Gang Leader (voice) |
 Pinto ColvigIchabod Crane (screaming) (voice) | Ichabod Crane (screaming) (voice) |
| LLeslie DenisonJudge / First Weasel (voice) | Judge / First Weasel (voice) |
| AAlec HarfordMr. Winky (voice) | Mr. Winky (voice) |
| EEdmond StevensSecond Weasel (voice) | Second Weasel (voice) |
 Billy BletcherHeadless Horseman (voice) | Headless Horseman (voice) |
| JJud ConlonTownsfolk (voice) (uncredited) | Townsfolk (voice) (uncredited) |
| MMack McLeanTownsfolk (voice) (uncredited) | Townsfolk (voice) (uncredited) |
 Clarence NashIchabod's Horse (voice) (uncredited) | Ichabod's Horse (voice) (uncredited) |
| LLoulie Jean NormanTownsfolk (voice) (uncredited) | Townsfolk (voice) (uncredited) |
| CCharlie ParlotaTownsfolk (voice) (uncredited) | Townsfolk (voice) (uncredited) |
| EEdmond StevensSecond Weasel (voice) (uncredited) | Second Weasel (voice) (uncredited) |
| OOliver WallaceMr. Winkie (voice) (uncredited) | Mr. Winkie (voice) (uncredited) |
 Gloria WoodTownsfolk (voice) (uncredited) | Townsfolk (voice) (uncredited) |
