 Burgess MeredithDr. Diabolo (Framing Story) | Dr. Diabolo (Framing Story) |
 Jack PalanceRonald Wyatt (segment 4 "The Man Who Collected Poe") | Ronald Wyatt (segment 4 "The Man Who Collected Poe") |
 Beverly AdamsCarla Hayes (segment 2 "Terror Over Hollywood") | Carla Hayes (segment 2 "Terror Over Hollywood") |
 Peter CushingLancelot Canning (segment 4 "The Man Who Collected Poe") | Lancelot Canning (segment 4 "The Man Who Collected Poe") |
 Maurice DenhamUncle Roger (segment 1 "Enoch") | Uncle Roger (segment 1 "Enoch") |
 Barbara EwingDorothy Endicott (segment 3 "Mr. Steinway") | Dorothy Endicott (segment 3 "Mr. Steinway") |
 Michael BryantColin Williams (segment 1 "Enoch") | Colin Williams (segment 1 "Enoch") |
 John StandingLeo Winston (segment 3 "Mr. Steinway") | Leo Winston (segment 3 "Mr. Steinway") |
 Robert HuttonBruce Benton (segment 2 "Terror Over Hollywood") | Bruce Benton (segment 2 "Terror Over Hollywood") |
 John PhillipsEddie Storm (segment 2 "Terror Over Hollywood") | Eddie Storm (segment 2 "Terror Over Hollywood") |
 Michael RipperGordon Roberts (Framing Story) | Gordon Roberts (Framing Story) |
 Bernard KayDr. Heim (segment 2 "Terror Over Hollywood") | Dr. Heim (segment 2 "Terror Over Hollywood") |
 Catherine FinnNurse Parker (segment 1 "Enoch") | Nurse Parker (segment 1 "Enoch") |
| UUrsula HowellsMiss Maxine Chambers (segment 3 "Mr. Steinway") | Miss Maxine Chambers (segment 3 "Mr. Steinway") |
 David BauerMike Charles (segment 2 "Terror Over Hollywood") | Mike Charles (segment 2 "Terror Over Hollywood") |
 Niall MacGinnisDr. Silversmith (segment 1 "Enoch") | Dr. Silversmith (segment 1 "Enoch") |
 Hedger WallaceEdgar Allan Poe(segment "4 "The Man Who Collected Poe"") | Edgar Allan Poe(segment "4 "The Man Who Collected Poe"") |
 Clytie JessopAtropos, Goddess of Destiny | Atropos, Goddess of Destiny |
