The men from U.N.C.L.E must stop a band of would-be sorcerers from using a deadly weapon.
| Actor | Role |
|---|---|
 Robert VaughnNapoleon Solo | Napoleon Solo |
 David McCallumIllya Kuryakin | Illya Kuryakin |
 Carol LynleyAnnie | Annie |
 Bradford DillmanLuther Sebastian | Luther Sebastian |
 Lola AlbrightAzalea | Azalea |
 Leo G. CarrollAlexander Waverly | Alexander Waverly |
 John DehnerDr. Kharmusi | Dr. Kharmusi |
 John CarradineThird-Way Priest | Third-Way Priest |
 Julie LondonLaurie Sebastian | Laurie Sebastian |
 H.M. WynantThe Aksoy Brothers | The Aksoy Brothers |
 Roy JensonCarl | Carl |
 Arthur MaletWhite Hunter | White Hunter |
 Robert KarnesShip's Captain | Ship's Captain |
 Barbara MooreLisa Rogers | Lisa Rogers |
 Kathleen FreemanMom | Mom |
 Sid HaigAlex | Alex |
 Lyzanne La DueWhite-Haired Girl | White-Haired Girl |
 Thordis BrandtMiss Zalamar | Miss Zalamar |