 Myron HealeyJohn Dillinger (archive footage) | John Dillinger (archive footage) |
 Paul DubovAlvin Karpis | Alvin Karpis |
 Sam EdwardsFred Barker | Fred Barker |
 Richard CraneHomer Van Meter | Homer Van Meter |
 Lyle TalbotDr. William Guellfe, Plastic Surgeon | Dr. William Guellfe, Plastic Surgeon |
 Jeanne CarmenPaula | Paula |
| TTamar CooperBonnie Parker | Bonnie Parker |
 Baynes BarronClyde Barrow | Clyde Barrow |
| DDoug WilsonCharles Arthur 'Pretty Boy' Floyd | Charles Arthur 'Pretty Boy' Floyd |
 Jim DavisPolice Captain Stewart / Narrator | Police Captain Stewart / Narrator |
| SSydney MasonLieutenant Bill Baxter | Lieutenant Bill Baxter |
 Lash LaRue'Doc' Barker | 'Doc' Barker |
 Ralph MoodyArthur 'Pa' Barker | Arthur 'Pa' Barker |
 Ann MorrissMildred Jaunce - The Lady in Red | Mildred Jaunce - The Lady in Red |
 Aline TowneShirley, Girl with Karpis | Shirley, Girl with Karpis |
| RRegina GleasonHope | Hope |
 Jeanne BatesMrs. Ross Baxter | Mrs. Ross Baxter |
| JJean Harvey'Ma' Barker (archive footage) | 'Ma' Barker (archive footage) |
| HHelen Van TuylTexas Lady Governor (archive footage) | Texas Lady Governor (archive footage) |
